A general and convenient procedure for the synthesis of N-alkylarylamines and N-alkylheteroarylamines by electrophilic amination of cuprates with N- …

P Bernardi, P Dembech, G Fabbri, A Ricci…

Index: Bernardi, Paolo; Dembech, Pasquale; Fabbri, Gaia; Ricci, Alfredo; Seconi, Giancarlo Journal of Organic Chemistry, 1999 , vol. 64, # 2 p. 641 - 643

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Citation Number: 53

Abstract

N-Alkylarylamines ArNHR can be prepared by the direct alkylation of primary aromatic amines with alkyl halides, 1 aryl sulfonates, 2 dialkyl phosphites, 3 or dimethyl oxalate, 4 provided that a large excess of the starting amine is used. However, the separation of the product from the reaction mixture is difficult. Tertiary N, N-(dialkyl) arylamines are invariably byproducts5 because the N-alkylarylamines produced in the first step are more ...

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