Catalyst-controlled regioselective Suzuki couplings at both positions of dihaloimidazoles, dihalooxazoles, and dihalothiazoles

NA Strotman, HR Chobanian, J He, Y Guo…

Index: Strotman, Neil A.; Chobanian, Harry R.; He, Jiafang; Guo, Yan; Dormer, Peter G.; Jones, Christina M.; Steves, Janelle E. Journal of Organic Chemistry, 2010 , vol. 75, # 5 p. 1733 - 1739

Full Text: HTML

Citation Number: 36

Abstract

Various dihaloazoles can be monoarylated at a single C− X bond with high selectivity via Suzuki coupling. By changing the palladium catalyst employed, the selectivity can be switched for some dihaloazoles, allowing for Suzuki coupling at the other, traditionally less reactive C− X bond. These conditions are applicable to coupling of a wide variety of aryl-, heteroaryl-, cyclopropyl-, and vinylboronic acids with high selectivities and enable the ...

Related Articles:

Environmental-benign oxidation of 2-oxazolines to oxazoles by dioxygen as the sole oxidant

[Huang, Yue; Ni, Lijun; Gan, Haifeng; He, Yu; Xu, Jinyi; Wu, Xiaoming; Yao, Hequan Tetrahedron, 2011 , vol. 67, # 11 p. 2066 - 2071]

… α-Oxo gold carbenes using bidentate ligands: implication of tricoordinated gold intermediates and the development of an expedient bimolecular assembly of 2, 4- …

[Luo, Yingdong; Ji, Kegong; Zhang, Liming; Li, Yuxue Journal of the American Chemical Society, 2012 , vol. 134, # 42 p. 17412 - 17415,4]

A domino copper-catalyzed CN and CO cross-coupling for the conversion of primary amides into oxazoles

[Schuh, Kerstin; Glorius, Frank Synthesis, 2007 , # 15 p. 2297 - 2306]

A novel improved procedure for the synthesis of oxazoles

[Huang, Wei; Pei, Jian; Chen, Bingzi; Pei, Weiwei; Ye, Xiulin Tetrahedron, 1996 , vol. 52, # 30 p. 10131 - 10136]

A domino copper-catalyzed CN and CO cross-coupling for the conversion of primary amides into oxazoles

[Schuh, Kerstin; Glorius, Frank Synthesis, 2007 , # 15 p. 2297 - 2306]

More Articles...