Tetrahedron Letters

Synthesis and ligation ability of mono-aminooxy-functionalized dendrigraft poly-l-lysine (DGL)

AM Bondia, N Larcher, L Garrelly, JC Rossi, R Pascal

Index: Bondia, Andrea Molero; Larcher, Nicolas; Garrelly, Laurent; Rossi, Jean Christophe; Pascal, Robert Tetrahedron Letters, 2010 , vol. 51, # 25 p. 3330 - 3333

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Citation Number: 4

Abstract

A bifunctional tetraethylene glycol (TEG) linker was prepared and used as an initiator for the synthesis of the first two generations of dendrigraft poly-l-lysines (DGL). The key steps involved the desymmetrization of TEG by introduction of an amine group after activation of a terminal hydroxyl group and of a conveniently protected aminooxy functionality at the other end. Initiation of l-lysine N-carboxyanhydride polymerization by the terminal amine yielded ...

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