A new approach to (S)-4-hydroxy-2-pyrrolidinone and its 3-substituted analogues

PQ Huang, X Zheng, SL Wang, JL Ye, LR Jin…

Index: Huang, Pei Qiang; Zheng, Xiao; Li Wang, Shi; Liang Ye, Jian; Ren Jin, Li; Chen, Zhong Tetrahedron Asymmetry, 1999 , vol. 10, # 17 p. 3309 - 3317

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Citation Number: 41

Abstract

Successive treatment of a phenyl thioether derived from (S)-malic acid with n-BuLi, lithium naphthalenide (LN), and electrophiles led to 4-hydroxy-3-substituted 2-pyrrolidinones in one- pot and in high regio-and diastereoselectivity at C-3. N-Debenzylation of 1-benzyl-4-hydroxy- 2-pyrrolidinone using LN afforded naturally occurring (−)-(S)-4-hydroxy-2-pyrrolidinone.(−)- (3S, 4S)-4-Hydroxy-3-methyl-2-pyrrolidinone, the lactam form of the γ-amino acid residue ...

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