Reaction of activated aryl and heteroaryl halides with hexamethylphosphoramide

JT Gupton, JP Idoux, G Baker, C Colon…

Index: Gupton, John T.; Idoux, John P; Baker, Graeme; Colon, Cesar; Crews, A.Donald; et al. Journal of Organic Chemistry, 1983 , vol. 48, # 17 p. 2933 - 2936

Full Text: HTML

Citation Number: 42

Abstract

good yield. The conversion of carboxylic acids to amides via HMPA has been previously reported5 in the literature. This experiment did, however, point out that acid amides were not suitable activating groups for such a reaction. Diary1 ketones, aryl alkyl ketones, and aromatic aldehydes (entries 1-n, Table I) were found to be unsuitable substrates for this reaction, and in these cases a complex mixture of products was formed. This is consistent ...

Related Articles:

A simple and efficient procedure for the Beckmann rearrangement of oxime using bis-(trichloromethyl) carbonate/DMF

[Su; Zhang; Li Organic Preparations and Procedures International, 2008 , vol. 40, # 6 p. 543 - 550]

One-pot conversion of aromatic bromides and aromatics into aromatic nitriles via aryllithiums and their DMF adduct

[Ushijima, Sousuke; Moriyama, Katsuhiko; Togo, Hideo Tetrahedron, 2011 , vol. 67, # 5 p. 958 - 964]

Direct transformation of N, N-disubstituted amides and isopropyl esters to nitriles

[Suzuki, Yusuke; Yoshino, Takumi; Moriyama, Katsuhiko; Togo, Hideo Tetrahedron, 2011 , vol. 67, # 21 p. 3809 - 3814]

Practical one-pot transformation of electron-rich aromatics into aromatic nitriles with molecular iodine and aq NH 3 using Vilsmeier–Haack reaction

[Ushijima, Sousuke; Moriyama, Katsuhiko; Togo, Hideo Tetrahedron, 2012 , vol. 68, # 24 p. 4588 - 4595]

Practical one-pot conversion of aryl bromides and β-bromostyrenes into aromatic nitriles and cinnamonitriles

[Ishii, Genki; Harigae, Ryo; Moriyama, Katsuhiko; Togo, Hideo Tetrahedron, 2013 , vol. 69, # 5 p. 1462 - 1469]

More Articles...