Tetrahedron

Imidazolylidenes, imidazolinylidenes and imidazolidines

AJ Arduengo, R Krafczyk, R Schmutzler, HA Craig…

Index: Arduengo III, Anthony J.; Krafczyk, Roland; Schmutzler, Reinhard; Craig, Hugh A.; Goerlich, Jens R.; Marshall, William J.; Unverzagt, Markus Tetrahedron, 1999 , vol. 55, # 51 p. 14523 - 14534

Full Text: HTML

Citation Number: 810

Abstract

Starting from glyoxal, 1, 3-diarylimidazolinium chlorides 3 were obtained in a three-step sequence via the diimines (1) and ethylene diamine dihydrochlorides (2). Reduction of 1, 3- diarylimidazolinium chlorides (3) with lithium alumnium hydride furnished the 1, 3- diarylimidazolidines (4) while their deprotonation with potassium hydride in thf gave access to stable carbenes (1, 3-diarylimidazolin-2-ylidenes, 5). Similarly substituted imidazol-2- ...

Related Articles:

A general and versatile approach to thermally generated N??heterocyclic carbenes

[Nyce, Gregory W.; Csihony, Szilard; Waymouth, Robert M.; Hedrick, James L. Chemistry - A European Journal, 2004 , vol. 10, # 16 p. 4073 - 4079]

A general and versatile approach to thermally generated N??heterocyclic carbenes

[Nyce, Gregory W.; Csihony, Szilard; Waymouth, Robert M.; Hedrick, James L. Chemistry - A European Journal, 2004 , vol. 10, # 16 p. 4073 - 4079]

A general and versatile approach to thermally generated N??heterocyclic carbenes

[Nyce, Gregory W.; Csihony, Szilard; Waymouth, Robert M.; Hedrick, James L. Chemistry - A European Journal, 2004 , vol. 10, # 16 p. 4073 - 4079]

Selective Reduction of Esters to Aldehydes under the Catalysis of Well??Defined NHC–Iron Complexes

[Li, Haoquan; Misal Castro, Luis C.; Zheng, Jianxia; Roisnel, Thierry; Dorcet, Vincent; Sortais, Jean-Baptiste; Darcel, Christophe Angewandte Chemie - International Edition, 2013 , vol. 52, # 31 p. 8045 - 8049 Angew. Chem., 2013 , vol. 125, # 31 p. 8203 - 8207]

Expanded ring diaminocarbene palladium complexes: synthesis, structure, and Suzuki–Miyaura cross-coupling of heteroaryl chlorides in water

[Kolychev, Eugene L.; Asachenko, Andrey F.; Dzhevakov, Pavel B.; Bush, Alexander A.; Shuntikov, Viacheslav V.; Khrustalev, Victor N.; Nechaev, Mikhail S. Dalton Transactions, 2013 , vol. 42, # 19 p. 6859 - 6866]

More Articles...