Tetrahedron

Synthesis of azafluorenones and related compounds using deprotocupration–aroylation followed by intramolecular direct arylation

N Marquise, PJ Harford, F Chevallier, T Roisnel…

Index: Marquise, Nada; Harford, Philip J.; Chevallier, Floris; Roisnel, Thierry; Dorcet, Vincent; Gagez, Anne-Laure; Sable, Sophie; Picot, Laurent; Thiery, Valerie; Wheatley, Andrew E.H.; Gros, Philippe C.; Mongin, Florence Tetrahedron, 2013 , vol. 69, # 47 p. 10123 - 10133

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Citation Number: 18

Abstract

Abstract The efficiency of the deprotocupration–aroylation of 2-chloropyridine using lithiocuprates prepared from CuX (X= Cl, Br) and LiTMP (TMP= 2, 2, 6, 6- tetramethylpiperidido, 2 equiv) was investigated. CuCl was identified as a more suitable copper source than CuBr for this purpose. Different diaryl ketones bearing a halogen at the 2 position of one of the aryl groups were synthesized in this way from azines and ...

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