A domino copper-catalyzed CO coupling-Claisen rearrangement process
G Nordmann, SL Buchwald
Index: Nordmann, Gero; Buchwald, Stephen L. Journal of the American Chemical Society, 2003 , vol. 125, # 17 p. 4978 - 4979
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Citation Number: 159
Abstract
A practical method for the diastereoselective generation of two adjacent quarternary stereocenters by combining a copper-catalyzed CO coupling reaction with a subsequent Claisen rearrangement in a one-pot domino process is described. Furthermore, an experimentally simple method for the stereoselective synthesis of a variety of different types of vinyl ethers is delineated using the same catalyst system.
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