Bulletin of the Chemical Society of Japan

An efficient and general method for the Reformatsky-type reaction of chlorodifluoromethyl ketones with carbonyl compounds giving. ALPHA.,. ALPHA.-difluoro-. BETA.- …

M Kuroboshi, T Ishihara

Index: Kuroboshi; Ishihara Bulletin of the Chemical Society of Japan, 1990 , vol. 63, # 2 p. 428 - 437

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Citation Number: 63

Abstract

Chlorodifluoromethyl ketones CF 2 ClCOR, where R is an alkyl, aryl, and 1-alkynyl group, underwent the Reformatsky-type aldol reaction with a wide variety of aldehydes or ketones in the presence of acid-washed zinc dust and copper (I) chloride or silver acetate to give the corresponding α, α-difluoro-β-hydroxy ketones in good to excellent yields. Specific activation of zinc metal with the metal salt is essential to achieve high efficiency of the reaction, ...

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