C–H cycloamination of N-aryl-2-aminopyridines and N-arylamidines catalyzed by an in situ generated hypervalent iodine (iii) reagent
Y He, J Huang, D Liang, L Liu, Q Zhu
Index: He, Yimiao; Huang, Jinbo; Liang, Dongdong; Liu, Lanying; Zhu, Qiang Chemical Communications, 2013 , vol. 49, # 66 p. 7352 - 7354
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Citation Number: 40
Abstract
A metal-free synthesis of diversified pyrido [1, 2-a] benzimidazoles and 1 H-benzo [d] imidazoles from N-aryl-2-aminopyridines and N-arylamidines has been developed. The C– H cycloamination reaction was catalyzed by hypervalent iodine (III) species generated in situ from iodobenzene (catalytic) and peracetic acid (stoichiometric). The reaction proceeded smoothly at ambient temperature to provide the corresponding N-heterocycles in good to ...
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