Lewis Acid-Mediated Michaelis− Arbuzov Reaction at Room Temperature: A Facile Preparation of Arylmethyl/Heteroarylmethyl Phosphonates

GG Rajeshwaran, M Nandakumar, R Sureshbabu…

Index: Rajeshwaran, Ganesan Gobi; Nandakumar, Meganathan; Sureshbabu, Radhakrishnan; Mohanakrishnan, Arasambattu K Organic Letters, 2011 , vol. 13, # 6 p. 1270 - 1273

Full Text: HTML

Citation Number: 64

Abstract

A facile preparation of arylmethyl and heteroarylmethyl phosphonate esters was achieved involving a Lewis acid mediated Michaelis− Arbuzov reaction at room temperature. Interaction of arylmethyl halides/alcohols with triethyl phosphite in the presence of Lewis acid at room temperature afforded phosphonate esters in good yields.

Related Articles:

A Novel Synthesis of Benzo [b] selenophenes via Regioselective Intramolecular Transformation of 4-(3-Nitroaryl)-1, 2, 3-selenadiazoles

[Makosza, Mieczyslaw; Sulikowski, Daniel Journal of Organic Chemistry, 2009 , vol. 74, # 10 p. 3827 - 3832]

A practical synthetic approach to chiral α-aryl substituted ethylphosphonates

[Goulioukina, Natalia S.; Dolgina, Tat'yana M.; Beletskaya, Irina P.; Henry, Jean-Christophe; Lavergne, Damien; Ratovelomanana-Vidal, Virginie; Genet, Jean-Pierre Tetrahedron Asymmetry, 2001 , vol. 12, # 2 p. 319 - 327]

Copper??Catalyzed Synthesis of Alkylphosphonates from H??Phosphonates and N??Tosylhydrazones

[Miao, Wenjun; Gao, Yuzhen; Li, Xueqin; Gao, Yuxing; Tang, Guo; Zhao, Yufen Advanced Synthesis and Catalysis, 2012 , vol. 354, # 14-15 p. 2659 - 2664]

Nucleophilic Alkylation of Carbenoids1; III. Copper (I)-Catalysed Replacement of the Chlorine Atoms in 1, 1-Dichloroalkanephosphonates by Various Substituents

[Villieras,J. et al. Synthesis, 1978 , p. 27 - 29]

Copper??Catalyzed Synthesis of Alkylphosphonates from H??Phosphonates and N??Tosylhydrazones

[Miao, Wenjun; Gao, Yuzhen; Li, Xueqin; Gao, Yuxing; Tang, Guo; Zhao, Yufen Advanced Synthesis and Catalysis, 2012 , vol. 354, # 14-15 p. 2659 - 2664]

More Articles...