Tetrahedron letters

Conversion of (1-heterodiene) tricarbonyliron (0) complexes into (2-aminohomodiene) tricarbonyliron (0) complexes

MJ Ackland, TN Danks, ME Howells

Index: Ackland, Mark J.; Danks, Timothy N.; Howells, Mark E. Tetrahedron Letters, 1996 , vol. 37, # 5 p. 691 - 694

Full Text: HTML

Citation Number: 11

Abstract

Treatment of (1-azadiene) tricarbonyliron (0) complex 1 with lithiated amines leads to attack at a metal carbonyl and the formation of formamides, whereas complexes 2 and 3 undergo deprotonation of the methyl group at C-2 followed by a rearrangement to form (2- aminohomodiene) tricarbonyliron (0) complexes 8 or 10 in good yield.

Related Articles:

SYNTHESIS OF SOME BENTROTRIAZOLES BY DEOXYGENATION OF O-NITROPHENYLAZO COMPOUNDS BY TERTIARY AMINES AND CO

[Gazzetta Chimica Italiana, , vol. 123, # 12 p. 683 - 686]

Preparation of Tertiary Amides from Carbamoyl Chlorides and Organocuprates

[Organic Letters, , vol. 6, # 21 p. 3703 - 3706]

Carbonylation of amines and diamines catalyzed by nickel carbonyl

[Martin, Wilbur E.; Farona, Michael F. Journal of Organometallic Chemistry, 1981 , vol. 206, # 3 p. 393 - 397]

Mild, simple, and efficient method for N-formylation of secondary amines via reimer–tiemann reaction

[Shastri, Lokesh A.; Shastri, Samundeeswari L.; Bathula, Chinna D.; Basanagouda, Mahantesha; Kulkarni, Manohar V. Synthetic Communications, 2011 , vol. 41, # 4 p. 476 - 484]

Well-defined iron catalyst for improved hydrogenation of carbon dioxide and bicarbonate

[Journal of the American Chemical Society, , vol. 134, # 51 p. 20701 - 20704]

More Articles...