Tetrahedron

One-pot synthesis of imidazolines from aldehydes: detailed study about solvents and substrates

H Fujioka, K Murai, O Kubo, Y Ohba, Y Kita

Index: Fujioka, Hiromichi; Murai, Kenichi; Kubo, Ozora; Ohba, Yusuke; Kita, Yasuyuki Tetrahedron, 2007 , vol. 63, # 3 p. 638 - 643

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Citation Number: 57

Abstract

Imidazolines were prepared in one-pot operation from aldehydes and diamines through oxidation of aminal intermediates by NBS. This method could be applied to various aromatic and aliphatic aldehydes and N-nonsubstituted and N-monosubstituted 1, 2-diamines. Furthermore, it was found that CH2Cl2 could be altered to TBME, a more environmentally friendly solvent, in the reaction using N-nonsubstituted 1, 2-diamines. The reaction ...

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