Abstract 2-Alkoxyiminoalkylmercaptans were treated with appropriate reagents by established procedures to prepare the corresponding “Bunte salts,” 2-(2- alkoxyiminoalkylthio)-2-imidazolines, 2-(2-alkoxyimino) alkyl dithiocarbonates, and ethyl 2- alkoxyiminoalkyl trithiocarbonates. Selected compounds were screened for radioprotective activity, and none was found to have significant activity.