The syntheses of many selenocarbonyl compounds have been reported and the recent reviews detail the studies. 1., , , , , , , and Selenoureas are used as the precursors for the syntheses of selenium–nitrogen heterocyclic compounds 2., , , , and and their activities have received increasing attentions. 3., , and There is only a few reports of preparation of N,N-unsubstituted selenourea by the reaction of hydrogen selenide with cyanamide. 2d The preparation of N,N- ...