A series of primary amido gallium alkyl complexes that includes a base free dimer,[t Bu 2Ga (μ-N (H) tBu)] 2 (1), Lewis base stabilized monomeric complexes, nBu2Ga (N (H) tBu)(THF)(2) and nBu2Ga [NH (2, 6-Me2C6H3)] py (3) and an anionic complex, nBu2Ga [NH (2, 6-Me2C6H3)] 2 [Li (Et2O)](4) is reported. Complex 1 crystallizes in the triclinic space group P-1 (a= 10.265 (5) A ̊, b= 15.752 (6) A ̊, c= 8.932 (4) A ̊, α= 90.32 (3)°, β= ...