The total synthesis of 5-(2′-hydroxyethyl) indolizidine via 5-thioindolizidinone is described. The key step is the transformation of 5-thioindolizidinone via Eschenmoser's sulfide contraction. The racemic mixture of 5R, 9R-and 5S, 9S-5-(2′-hydroxyethyl) indolizidine was obtained in seven steps in 17% overall yield from 2-allyl cyclopentanone.
[Crandall, Jack K.; Magaha, H. Steve; Henderson, Mark A.; Widener, Rexford K.; Tharp, Gregg A. Journal of Organic Chemistry, 1982 , vol. 47, # 27 p. 5372 - 5380]
[Pearson, William H.; Walavalkar, Rajesh; Schkeryantz, Jeffrey M.; Fang, Wen-Kui; Blickensdorf, James D. Journal of the American Chemical Society, 1993 , vol. 115, # 22 p. 10183 - 10194]
[Pearson, William H.; Walavalkar, Rajesh; Schkeryantz, Jeffrey M.; Fang, Wen-Kui; Blickensdorf, James D. Journal of the American Chemical Society, 1993 , vol. 115, # 22 p. 10183 - 10194]