The direct amination of C¿ H bonds is a unique synthetic approach towards the important class of alkylated nitrogen compounds.[1] In this context, the palladium-catalyzed intermolecular C (sp3)¿ H activation/amination of alkyl groups is a notably unexplored process.[2–4] On the other hand, we recently came across a reaction based on the formation of alkyl–nitrogen bonds from s-alkyl palladium intermediates in the context of developing ...