Several fused aromatic tetracyanep-quincdimethane (TCNQ) derivatives (lla-c, 5, and 12) have been synthesized by the reaction of the corresponding quinones and malononitrile. Syntheses of these derivatives by Diels-Alder reactions of o-quinodimethane and TCNQ have been attempted. In comparison with TCNQ, cyclic voltammetric data of these new compounds reveal a more negative value for the first and the second reduction potential.